If you want more kinds of small caps, you might apply the FakeBold feature to a different weight, or you might find this code useful. \makebox does nothing and Ligatures = NoDiscretionary only produces a second error message saying that the font does not support dlig. The short answer is: the day in 1861 when Italy unified and acquired an army and a navy. Latin shares only between 25-35 percent of its basic vocabulary with such languages as Gothic, Vedic Sanskrit, old Irish, and Old Armenian, showing that there was a long period of separation between Latin and the rest of these.
The macros \textbfsl and \textbfslsc are for now very naive approaches to do this, unbreakable text, but I hope that enough to check is it could look like true bold fonts (sorry again, but now I do not have time to test a more handy approach to overlap text, maybe later): It is because we don’t call Italian as Modern Latin like we call the language spoken in Greece today as Modern Greek. Latin vocabulary is mostly Italic in origin, however, some frequent Latin words have no Italic etymology, e.g., mulier ‘woman’, bonus ‘good’. Other is botch with one has available: Using pdflatex you can simulate "Italics smallcaps" with "Slanted smallcaps" using slantsc packages, at least with pdflatex (not tested with lualatex, sorry) and the simulate the bold variant overlaping text. One approach to solve this could be change the Latin Modern by another font with enough glyphs (I do not know a free font with enough glyphs, but probably a professional font could cover all your desired styles). As fas I know, there are not any good solution for this. Changing default font typeface Computer Modern (default in standard LaTeX classes): CM Roman, CM Sans Serif, CM Typewriter Latin Modern: LM Roman, LM Sans.
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